4.6 Article

Influence of optically quenched superconductivity on quasiparticle relaxation rates in Bi2Sr2CaCu2O8+δ

Journal

PHYSICAL REVIEW B
Volume 92, Issue 16, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.92.161102

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Funding

  1. Ultrafast Materials Program at Lawrence Berkeley National Laboratory - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]

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We use time- and angle-resolved photoemission to measure quasiparticle relaxation dynamics across a laser-induced superconducting phase transition in Bi2Sr2CaCu2O8+delta . Whereas low-fluence measurements reveal picosecond dynamics, sharp femtosecond dynamics emerge at higher fluence. Analyses of data as a function of energy, momentum, and doping indicate that the closure of the near-nodal gap and disruption of macroscopic coherence are primarymechanisms driving this onset. The results demonstrate the important influence of transient electronic structure on relaxation dynamics, which is relevant for developing an understanding of nonequilibrium phase transitions.

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