4.6 Article

Graphene in ultrafast and superstrong laser fields

Journal

PHYSICAL REVIEW B
Volume 91, Issue 4, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.91.045439

Keywords

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Funding

  1. Chemical Sciences, Biosciences and Geosciences Division [DE-FG02-01ER15213]
  2. Materials Sciences and Engineering Division of the Office of the Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-11ER46789]
  3. NSF [ECCS-1308473]
  4. Max Planck Society
  5. Deutsche Forschungsgemeinschaft Cluster of Excellence: Munich Center for Advanced Photonics
  6. Div Of Electrical, Commun & Cyber Sys
  7. Directorate For Engineering [1308473] Funding Source: National Science Foundation

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For graphene interacting with a few-fs intense optical pulse, we predict unique and rich behavior dramatically different from three-dimensional solids. Quantum electron dynamics is shown to be coherent but highly nonadiabatic and effectively irreversible due to strong dephasing. Electron distribution in reciprocal space exhibits hot spots at the Dirac points and oscillations whose period is determined by nonlocality of electron response and whose number is proportional to the field amplitude. The optical pulse causes net charge transfer in the plane pf graphene in the direction of the instantaneous field maximum at relatively low fields and in the opposite direction at high fields. These phenomena promise ultrafast optoelectronic applications with petahertz bandwidth.

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