Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 83, Issue 17, Pages 10080-10088Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.8b01393
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Funding
- National Program on Key Research Project [2016YFA0602900]
- National Natural Science Foundation of China [21572068]
- Science and Technology Program of Guangzhou, China [201707010057]
- Guangdong Natural Science Foundation [2017A030312005]
- Science and Technology Planning Project of Guangdong Province, China [2017A020216021]
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Unsaturated N,O-spiroacetals and alpha-arylfurans were synthesized via palladium-catalyzed aerobic oxidative coupling reactions between N-[3-(2-furanyl)propyl]-p-toluenesulfonamides and boronic acids, with KF and KOAc as the respective additives. These reactions involve an unprecedented dearomatizing 2,5-aminoarylation and a direct alpha-arylation of furan rings, respectively, with O-2 as the terminal oxidant.
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