Journal
PHYSICAL REVIEW A
Volume 91, Issue 5, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.91.053424
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Funding
- ERC-AdG [320459]
- EPSRC [EP/L005913/1]
- EU through grant FP7 ITN ICONIC [238671]
- STFC through mini-IPS grant [ST/J002895/1]
- ISIS Innovation Ltd.
- DFG [LA 3209/1-1, LA 3209/1-2]
- STFC through a PNPAS award
- EPSRC [EP/L005913/1] Funding Source: UKRI
- STFC [ST/J002895/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/L005913/1] Funding Source: researchfish
- Science and Technology Facilities Council [ST/J002895/1] Funding Source: researchfish
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Femtosecond laser-induced Coulomb-explosion imaging of 3,5-dibromo- 3',5'-difluoro-4'-cyanobiphenyl molecules prealigned in space is explored using a pixel-imaging mass-spectrometry (PImMS) camera. The fast-event-triggered camera allows the concurrent detection of the correlated two-dimensional momentum images, or covariance maps, of all the ionic fragments resulting from fragmentation of multiple molecules in each acquisition cycle. Detailed simulation of the covariance maps reveals that they provide rich information about the parent molecular structure and fragmentation dynamics. Future opportunities for imaging the real-time dynamics of intramolecular processes are considered.
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