Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 79, Issue 4, Pages 1867-1871Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo402778p
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Funding
- National Science Foundation of China [21202049]
- Recruitment Program of Global Experts (1000 Talents Plan)
- Fujian Hundred Talents Program
- Research Funds of Huaqiao University
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Aromatic aldehydes or ketones from copper catalyzed aerobic oxidative decarboxylation of phenylacetic acids and alpha-hydroxyphenylacetic acids have been synthesized. This reaction combined decarboxylation, dioxygen activation, and C-H bond oxidation steps in a one-pot protocol with molecular oxygen as the sole terminal oxidant. This reaction represents a novel decarboxylation of an sp(3)-hybridized carbon and the use of a benzylic carboxylic acid as a source of carbonyl compounds.
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