Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 78, Issue 18, Pages 9120-9126Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo401324k
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Funding
- National Natural Science Foundation of China [20872127, J0830431]
- National Basic Research Program of China (973 Program) [2009CB825300]
- CAS Academician Foundation of Zhejiang Province
- Fundamental Research Funds for the Central Universities
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A gold-catalyzed cyclization of 3-(2'-azidoaryl)-1-arylpropargyl carbonates to generate substituted quinolines via a sequence of 3,3-rearrangement, 6-endo-trig cyclization and denitrogenation has been developed. Similar products could be obtained from 3-aryl-1-(2'-azidoaryl)propargyl carbonates under different gold catalytic conditions via a sequential 6-endo-dig cyclization, denitrogenation, and 1,2-H shift process.
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