Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 78, Issue 19, Pages 9969-9974Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo4013783
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Funding
- The National Institutes of Health [GM087981]
- The Robert A. Welch Foundation [A-1121]
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Imidazolinylidene, imidazolylidine, benzimidazolylidene complexes 1a-c were prepared and tested in asymmetric hydrogenations of a series of largely unfunctionalized alkenes. Similarities and differences in the catalytic performance of these complexes were rationalized in terms of the predicted mechanisms of these reactions, and their relative tendencies to generate protons under the hydrogenation conditions.
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