Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 77, Issue 8, Pages 4143-4147Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo3002535
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Funding
- National Natural Foundation of China
- Ministry of Science and Technology [2011CB808600]
- Chinese Academy of Sciences
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A Me-DuPhos-catalyzed efficient asymmetric [3 + 2] cycloaddition reaction between Morita-Baylis-Hillman carbonates of isatins and N-phenylmaleimide has been developed. This reaction constructs three chiral centers in one step to afford spirocyclopentaneoxindoles in good yields (up to 84%) with excellent diastereo- and enantioselectivies (up to 99% ee).
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