Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 77, Issue 6, Pages 2942-2946Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo2024812
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Funding
- National Natural Science Foundation of China [20806012, 20972022]
- Ministry of Education of China
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With the direct use of allylic alcohols as allylating agents, the Friedel Crafts-type allylic alkylation of nitrogen-containing aromatic compounds catalyzed by a [Mo3S4Pd(eta(3)-allyl)] cluster is achieved. With a 3 mol % catalyst loading in acetonitrile at re lux or 60 degrees C, a variety of N,N-dialkylanilines and indoles reacted smoothly with allylic alcohols to afford the Friedel-Crafts-type allylation products in good to excellent yields with high levels of regioselectivity.
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