Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 75, Issue 23, Pages 8279-8282Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo101554r
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Funding
- National Natural Science Foundation of China [20625205, 20772034, 20932002]
- National Basic Research Program of China (973 Program) [2011CB808603]
- Ministry of Education of China [20090172110014]
- Guangdong Natural Science Foundation [1035106410-1000000]
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A palladium-catalyzed 1:2 linear/cyclic cross-trimerization of alkyne with alkenes using molecular oxygen as the sole oxidant has been reported for the first time. A series of 1,3,5-trienes and 1,2,4,5-tetrasubstituted benzenes are obtained with high chemoselectivity respectively and mechanisms of these reactions are proposed based on some controlled examination.
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