Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 75, Issue 7, Pages 2403-2406Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo902500b
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Funding
- National Science Foundation of China [20872004]
- Shenzhen municipal Shuang Bai Project
- Shenzhen Bureau of Science and Technology
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The Mannich reactions previously extensively investigated with organocatalysis of L-proline and other related small molecules were reinvestigated with detailed stercochemical analysis of their autocatalysis pathways, through employment of both the products themselves and their close structural mimics as the catalysts. These organo-autocatalytic processes function as meaningful molecular models toward understanding the origin and maintenance of homochirality under biologically relevant conditions.
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