Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 74, Issue 24, Pages 9486-9489Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo902204s
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Funding
- National Science Foundation of China [20672090, 20810102050, 20928001]
- Natural Science Foundation of the Jiangsu Province [BK2006033]
- Six Kinds of Professional Elite Foundation of the Jiangsu Province [06-A-039]
- Qing Lan Project [08QLT001]
- National Institutes of Health [R03DA026960]
- Robert A. Welch Foundation [D-1361]
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Concise and efficient six-component and four-component domino approaches to anti-1,2-diarylethylbenzamides and highly Substituted 2-(2'-azaaryl)imidazoles have been developed under solvent-free and microwave-irradiation conditions. The reactions showed a broad scope of substrates in which a wide range of common commercial aromatic aldehydes and heteroaryl nitriles can be used. The syntheses were Finished within short periods (15-34 min) with good to excellent chemical yields and stereoselectivity that avoided tedious workup isolations. New mechanisms involving an umpolung have been proposed for these two reaction processes.
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