Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 73, Issue 11, Pages 4225-4228Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo800203d
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Three novel boomerang precatalysts bearing different aminocarbonyl functions are reported. Comparative kinetic studies show that this functional group allows for a control of the catalytic activity in metathesis transformations. The scope of the more active catalyst is investigated and shows a good tolerance to various substrates in ring-closing metathesis, enyne metathesis, and cross metathesis. ICP-MS analyses illustrate the good affinity of this catalyst for silica gel, as levels of Ru contamination lower than 6 ppm are detected in the final products.
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