Journal
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES
Volume 373, Issue 2044, Pages -Publisher
ROYAL SOC
DOI: 10.1098/rsta.2014.0323
Keywords
singlet fission; tetracene; magnetic field effect
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Funding
- Center for Excitonics, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001088]
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Magnetic field effects provide a convenient and specific probe of singlet exciton fission within optoelectronic devices. Here, we demonstrate that this tool may also be applied to screen potential fission material candidates in solution. We characterize the phenomenon in diphenyl tetracene (DPT), which shows strong fluorescence modulation and the expected field dependence in its transient decay as a function of concentration. Solution measurements may also be used to test for the presence of an intermediate charge transfer state, but we observe no changes to the field dependence of DPT singlet exciton fission in toluene relative to chloroform.
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