Journal
JOURNAL OF NATURAL GAS CHEMISTRY
Volume 19, Issue 1, Pages 91-95Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S1003-9953(09)60032-3
Keywords
sulfur recovery; Co-Mo catalyst; carbon nanotubes; HDS process
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Effects of carbon nanotubes (CNT) and alumina (gamma-Al2O3) Supports on the catalytic activities of hydrodesulfurization (HDS) process over Co-Mo catalyst have been studied. XRD results indicated that the main active phases in CNT and gamma-Al2O3 supported Co-Mo catalysts are MoO2 and MoO3, respectively. The TPR results reveal that the reduction peak temperatures of the active species on CNT supported Co-Mo catalyst is lower than those on alumina supported Co-Mo catalyst, indicating that the CNT supports favor the reduction of active species. Catalytic evaluation results displayed that the sulfur content in the reaction products on the CNT supported Co-Mo catalyst is lower than that on the alumina supported Co-Mo catalyst if the HDS reaction was carried out at a temperature above 583 K.
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