4.3 Article

Laser-induced nonsequential double ionization: kinematic constraints for the recollision-excitation-tunneling mechanism

Journal

JOURNAL OF MODERN OPTICS
Volume 57, Issue 11, Pages 984-991

Publisher

TAYLOR & FRANCIS LTD
DOI: 10.1080/09500340903414619

Keywords

nonsequential double ionization; excitation; electron-electron correlation

Categories

Funding

  1. UK EPSRC [EP/D07309X/1]
  2. EPSRC [EP/D07309X/1, EP/D07309X/2] Funding Source: UKRI
  3. Engineering and Physical Sciences Research Council [EP/D07309X/1, EP/D07309X/2] Funding Source: researchfish

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We investigate the physical processes in which an electron, upon return to its parent ion, promotes a second electron to an excited state, from which it subsequently tunnels. Employing the strong-field approximation and saddle-point methods, we perform a detailed analysis of the dynamics of the two electrons, in terms of quantum orbits, and delimit constraints for their momentum components parallel to the laser-field polarization. The kinetic energy of the first electron, upon return, exhibits a cutoff slightly lower than 10U(p), where U-p is the ponderomotive energy, as in rescattered above-threshold ionization (ATI). The second electron leaves the excited state in a direct ATI-like process, with the maximal energy of 2U(p). We also compute electron-momentum distributions, whose maxima agree with our estimates and with other methods.

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