Journal
JOURNAL OF MEMBRANE SCIENCE
Volume 564, Issue -, Pages 813-819Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.memsci.2018.07.087
Keywords
Graphene oxide; Nanofiltration; Interfacial polymerization; Water transport; Ionic sieving
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Funding
- Natural Science Foundation of Beijing Municipality [2172027]
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Membranes with high permeability and selectivity are desired for energy-efficient liquid separation. In the present work, a highly wrinkled surface and ultrafast water transport channels centered in a graphene oxide (GO)-in-polyamide membrane were prepared by in-situ embedding GO nanosheets into the separation layer of a nanofiltration (NF) membrane via an interfacial polymerization. The rough and hydrophilic surface enabled the attraction of large amounts of water molecules to the membrane, and the sub-20 nm membrane thickness and two-dimensional capillary network formed by the stacked GO nanosheets accelerated the transport of water molecules through the membrane. This wrinkled and sandwich structured ultrathin NF composite membrane gave a water flux up to 242 LMH/MPa (nearly four-fold higher than those of reported NF membranes) and an unchanged high salt rejection, simultaneously.
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