Extending potential flow modelling of flat-sheet geometries as applied in membrane-based systems

The efficiency of chemical reactors can be analysed using the residence time distribution. This research focusses on flat-sheet geometries applied in membrane-based systems. The residence time distribution depends mainly on the 2D velocity field, parallel to the membrane. The velocity average over the transversal direction is calculated using potential flow theory. A combination of real and virtual sources and sinks are used to model the internal inlets and outlets. Furthermore, a novel method is presented to calculate the residence time distribution. By ignoring diffusion and dispersion, every streamline is modelled to have a fixed residence time, which can be calculated with a simple quadrature based on a coordinate transformation. The model predicts the impact of the two-dimensional geometry on the residence time distribution, but it is demonstrated that large zones of nearly stagnant flow have only a limited impact on the residence time distribution. The new model can predict the travelling time from the inlet to each interior location, providing a better tool to analyse spatially distributed chemical reactions. The models agreed highly with pressure measurements (R-2 = 0.94-0.98) and they agreed well with tracer experiments for the residence time (R-2 = 0.73-0.99). (C) 2008 Elsevier B.V. All rights reserved.