Journal
JOURNAL OF MATERIALS RESEARCH
Volume 28, Issue 7, Pages 958-968Publisher
CAMBRIDGE UNIV PRESS
DOI: 10.1557/jmr.2012.413
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Funding
- CMMI Division of the National Science Foundation [0800680]
- Materials Research Science and Engineering Center (NSF-MRSEC) on Polymers [0213695]
- Nanoscale Science and Engineering Center (NSF-NSEC) on hierarchical manufacturing [0531171]
- University of California, Riverside
- American Public Power Association DEED fellowship program
- Directorate For Engineering [0800680] Funding Source: National Science Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [0213695] Funding Source: National Science Foundation
- Div Of Civil, Mechanical, & Manufact Inn [0800680] Funding Source: National Science Foundation
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We report on the successful synthesis of a graphene-carbon nanotube (CNT) hybrid architecture by a parallel chemical vapor deposition (CVD) of the two carbon allotropes. The carbon hybrid is a three-dimensional (3D) nanostructure with tuneable architecture comprising vertically grown CNTs as pillars and a large-area graphene plane as the floor. The formation of CNTs and graphene occurs simultaneously in a single CVD growth that we describe as a synchronous synthesis method. Unique nature of the fabrication approach contributes significantly to the quality and composure of final nanohybrid. Detailed characterization elucidates the cohesive structure and robust contact between the graphene floor and the CNTs in the hybrid structure. The functionality of the synthesized graphene hybrid structure has been demonstrated by its incorporation into a super-capacitor cell. Our fabrication approach provides an attractive pathway for the fabrication of novel 3D hybrid nanostructures and efficient device integration.
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