Journal
JOURNAL OF MATERIALS CHEMISTRY
Volume 22, Issue 15, Pages 7456-7460Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2jm30442b
Keywords
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Funding
- National Natural Science Foundation of China [51073147]
- National Basic Research Program of China [2010CB923302, 2011CB921403]
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Metal-free catalysts are essential for various chemical reactions in industrial chemistry. Amino-functionalized carbon is a cheap and environmentally friendly solid basic catalyst. Here, NEt3-graphene solid basic catalyst has been synthesized through a consecutive deprotonation/carbometalation and electrophilic substituent. Transmission electron microscopy (TEM), scanning electron microscopy (SEM), elemental analyses, thermal analyses, Raman spectroscopy, and X-ray photoelectron spectroscopy (XPS) studies confirmed the formation of the target structure. Catalytic hydrolysis of ethyl acetate reveals that the amino-grafted graphene has a high catalytic activity.
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