Journal
JOURNAL OF MATERIALS CHEMISTRY
Volume 22, Issue 33, Pages 16986-16993Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2jm32841k
Keywords
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Funding
- Fundamental R&D Program for Technology of World Premier Materials
- Ministry of Knowledge Economy, Republic of Korea
- National Research Foundation of Korea (NRF)
- Korea Government (MEST) [2011-0029865]
- National Research Foundation of Korea [2010-0029244] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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The battery-supercapacitor hybrid electrode, consisting of both faradaic rechargeable battery components and non-faradaic rechargeable supercapacitor components in a single electrode, is successfully developed using Li4Ti5O12-activated carbon (LTO-AC) hybrid nanotubes in a negative electrode for an advanced energy storage device. Li4Ti5O12 and PVA-derived activated carbon are hybridized with morphological control over the one-dimensional (1D) tubular structures via an in situ sol-gel reaction combined with electrospinning, followed by a hydrothermal reaction and appropriate heat treatment. The prepared LTO-AC hybrid nanotubes are tested at a variety of charge-discharge rates as anode materials for use in lithium-ion rechargeable batteries that deliver a specific capacity in the range of 128-84 mA h g(-1) over a 100-4000 mA g(-1) charge-discharge rate in the potential range 1.0-2.5 V vs. Li/Li+. The hybridized LTO-AC hybrid nanotubes electrode is included in a new type of hybrid energy storage cell, denoted as BatCap, as the negative electrode using commercialized activated carbon (AC) as the positive electrode. The hybrid BatCap cell exhibits a high energy density of 32 W h kg(-1) and a high power density of 6000 W kg(-1), comparable to the properties of a typical AC symmetric capacitor.
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