Journal
JOURNAL OF MATERIALS CHEMISTRY
Volume 22, Issue 30, Pages 15141-15145Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2jm32354k
Keywords
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Funding
- National Research Foundation of Korea (NRF)
- Center for Advanced Soft Electronics under the Global Frontier Research
- Ministry of Education, Science and Technology [2009-0084786, 2012-0000127, 2011-0031639]
- National Research Foundation of Korea [2009-0084786] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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A conjugated polymer donor material, poly(3,4'''-di(decylthiophenyl) quaterthiophene) (PDTQT), featuring decylthiophenyl side chains on the polymer backbone, was introduced to reduce the crystallinity of poly(quaterthiophene) (PQT-C12) layers in organic photovoltaic cells. The resulting PDTQT: PC71BM blend active layer formed a well-interpenetrated nanoscale morphology that increased the power conversion efficiency (PCE) relative to devices based on highly crystalline PQT-C12. Bulk heterojunction solar cells fabricated using the PDTQT: PC71BM blend thin films yielded the best photovoltaic performances with a high short-circuit current density of 9.8 mA cm(-2), a high open-circuit voltage of 0.91 V, a fill factor of 0.36, and a high PCE of 3.2% under AM 1.5G illumination with an intensity of 100mW cm(-2). Decylthiophenyl side chain substitution appeared to be an effective strategy for obtaining high organic photovoltaic cell device performances.
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