Journal
JOURNAL OF MATERIALS CHEMISTRY
Volume 21, Issue 10, Pages 3359-3364Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0jm02852e
Keywords
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Funding
- National Natural Science Foundation of China [50972101]
- Guangdong-CAS [2009B091300007]
- Foundation of State Key Laboratory of Coal Conversion [10-11-913]
- Program for New Century Excellent Talents in University [NCET-07-0607]
- Ministry of Education, China
- Program of Introducing Talents of Discipline to Universities, China [B06006]
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Free-standing graphene-based macroscopic membranes, which are characterized by a layered structure and tunable conductivity, are prepared by a self-assembly process at a liquid-air interface. Since the preliminary results indicate that it is hard to construct macroscopic graphene membranes solely by low-temperature exfoliated graphene nanosheets (LGNs) at the liquid-air interface, graphene oxide nanosheets (GONs), as the stacking template and sticking component, are introduced into the assembly process of graphene layers to promote the formation of layer-by-layer stacking structure and help form a conductive macroscopic membrane. The conductivity of such a graphene-based membrane can be tuned by changing the GON fraction in the LGN/GON hybrid membrane.
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