Journal
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
Volume 335, Issue -, Pages 101-104Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jmmm.2013.01.043
Keywords
Half-metallicity; Heusler alloy; Anisotropy magnetoresistance
Funding
- National Natural Science Foundation of China [51071172, 51171207]
- National Basic Research Program of China (973 Programs) [2012CB619405]
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In this paper, we investigate the half-metallicity of Heusler alloys Fe2Co1-x CrxSi by first principles calculations and anisotropy magnetoresistance measurements. It is found that, with the increase of Cr content x, the Fermi level of Fe2Co1-xCrxSi moves from the top of valence band to the bottom of conduction band, and a large half-metallic band gap of 0.75 eV is obtained for x=0.75. We then successfully synthesized a series of Heusler Fe2Co1-x CrxSi polycrystalline ribbon samples. The results of X-ray diffraction indicate that the Fe2Co1-x CrxSi series of samples are pure phase with a high degree of order and the saturation magnetic moment follows half-metallic Slater-Pauling rule. Except for the two end members, Fe2CoSi and Fe2CrSi, the anisotropic magnetoresistance of Fe2Co1-x CrxSi (x=0.25, 0.5, and 0.75) shows a negative value suggesting they are stable half-metallic ferromagnets. (C) 2013 Elsevier B.V. All rights reserved.
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