Journal
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
Volume 18, Issue 2, Pages 808-813Publisher
ELSEVIER SCIENCE INC
DOI: 10.1016/j.jiec.2011.10.006
Keywords
Oxidative dehydrogenation; n-Butane; Oxygen mobility; Oxygen capacity; Vanadium-magnesium oxide
Funding
- Samsung Total Petrochemicals Corporation
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Vanadium-magnesium oxide (Mg-3(VO4)(2)) catalysts supported on Al2O3, ZrO2, MgO, and CeO2 were prepared by a wet impregnation method, and they were applied to the oxidative dehydrogenation of n-butane. Effect of oxygen capacity and oxygen mobility of supported Mg-3(VO4)(2) catalysts on the catalytic performance in the oxidative dehydrogenation of n-butane was investigated. Experimental results revealed that large oxygen capacity of the catalyst was favorable for obtaining high catalytic activity at the initial stage of reaction, while facile oxygen mobility of the catalyst led to stable catalytic activity during the catalytic reaction in the oxidative dehydrogenation of n-butane. (C) 2011 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
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