Journal
ORGANIC LETTERS
Volume 17, Issue 21, Pages 5360-5363Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b02717
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Funding
- National Nature Science Foundation of China [21372011, 21402001, 21472002]
- Nature Science Foundation of Anhui Province [1508085J07]
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A set of highly stable conformation-restricted partially and fully fused BODIPY dimers (alpha,beta-cyclohexadiene-fused and alpha,beta-benzene-fused dimers) were synthesized from a one-pot condensation of 2-formylpyrroles with alpha,beta-cydohexadiene-fused bipyrrole 3. Effective expansion of pi-conjugation over these fused BODIPY dimers was observed by X-ray analysis, density functional theory (DFT) calculations, and electrochemical and optical measurements, as demonstrated by their strong absorption and emissions in the near-infrared (NIR) range (650 to 820 nm).
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