Journal
ORGANIC LETTERS
Volume 18, Issue 1, Pages 128-131Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03317
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Funding
- National Natural Science Foundation of China [21202143, 21472163]
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A novel Fe-catalyzed olefin hydroamination with diazo compounds for accessing hydrazones has been developed. Diazo compounds are used as radical acceptors and can be trapped by the in situ generated alkyl radical toward C-N bond formation. The reaction conditions are mild, and the substrate scope is broad. Additionally, this hydroamination protocol is applicable for intramolecular reactions to construct diverse heterocycles.
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