Journal
ORGANIC LETTERS
Volume 17, Issue 24, Pages 6066-6069Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03047
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Funding
- National Science Foundation under the CCI Center for Selective C-H Functionalization [CHE-1205646]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1205646] Funding Source: National Science Foundation
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A comparative study is disclosed that seeks to highlight the current limitations and challenges that exist in the field of atom-transfer C-H oxidations. State-of-the-art methods are benchmarked in order to showcase clear differences and similarities. A novel Mn-mediated method for C-H oxidation is disclosed that serves as a rapid and simple method for aliphatic C-H hydroxylation. Finally, two methods that allow for C-H oxidation in the presence of pyridine-containing substrates are studied, something that is rare in the field but of great interest to the chemical community.
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