Journal
ORGANIC ELECTRONICS
Volume 22, Issue -, Pages 154-159Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.orgel.2015.03.053
Keywords
Phosphorescent organic light-emitting diodes; Gold nanoparticle; Surface plasmons
Funding
- Natural Science Foundation of China [61205025]
- Research Grants Council of Hong Kong Special Administrative Region, China [T23-713/11]
- Hong Kong Baptist University Strategic Development Fund [SDF13-0531-A02]
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Enhanced efficiency and reduced efficiency roll-off in phosphorescent organic light-emitting diodes (PhOLEDs) are realized by interposing a solution-processed gold nanoparticle (GNP)-based interlayer between the anode and the hole-injection layer. Transient photoluminescence measurements elucidate that a reduced lifetime of the triplet excitons was observed for samples having a GNP-interlayer as compared to a control sample without the GNP-interlayer. The decrease in the triplet exciton lifetime, caused by the coupling between the triplet excitons and the localized surface plasmons (LSPs) excited by the GNPs, enables reducing the triplet-triplet and triplet-polaron annihilation processes, thereby a reduced efficiency roll-off in PhOLEDs. The presence of a GNP-interlayer also acts as an optical out-coupling layer contributing to the efficiency enhancement and was demonstrated by the theoretical simulation. (C) 2015 Elsevier B.V. All rights reserved.
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