Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 13, Issue 47, Pages 11561-11566Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ob01763g
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Funding
- National Science Foundation of China [21202093, 21472112]
- Program for New Century Excellent Talents in University [NCET-13-0346]
- Shandong Science Fund for Distinguished Young Scholars [JQ201404]
- Young Scientist Foundation Grant of Shandong Province [BS2013YY001]
- Fundamental Research Funds of Shandong University [2014JC005, 2015JC035]
- Key Laboratory for the Chemistry and Molecular Engineering of Medicinal Resources (Guangxi Normal University), the Ministry of Education of China [CHEMR2014-B11]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT13028]
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An effective and metal-free oxidative cross-dehydrogenative coupling (CDC) of N-heterocycles with diverse aldehydes has been established in the presence of TBHP/TFA. The scope with respect to aldehyde and N-heterocycle components is broad, allowing facile synthesis of a broad range of structurally diverse C-1-acyl substituted heterocycles in good efficiency.
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