Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 13, Issue 26, Pages 7154-7158Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ob00781j
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Funding
- NSFC [21162025, 21262035]
- Program for Outstanding Youth Science and Technology Innovation Talents Training in Xinjiang Uygur Autonomous Region [2014721004]
- Natural Science Foundation of Xinjiang University [BS110133]
- Key Laboratory of Oil & Gas Fine Chemicals, Ministry of Education & Xinjiang Uyghur Autonomous Region [XJDX0908-2013-1, XJDX0908-2013-2]
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The heterocyclic ionic liquid-catalyzed direct oxidative amination of benzylic sp(3) C-H bonds via intermolecular sp(3) C-N bond formation for the synthesis of N-alkylated azoles under metal-free conditions is reported for the first time. The catalyst 1-butylpyridinium iodide can be recycled and reused with similar efficacies for at least eight cycles.
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