Journal
JOURNAL OF HAZARDOUS MATERIALS
Volume 159, Issue 2-3, Pages 587-592Publisher
ELSEVIER
DOI: 10.1016/j.jhazmat.2008.02.061
Keywords
Advanced oxidation processes; Catalytic ozonation; Phenol; Brucite; Magnesia
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Funding
- National Natural Science Foundation of China [50474036, 20673056]
- Environmental Protecting Science Foundation of Jiangsu Province [2007016]
- Open Analysis Foundation of Nanjing University
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Natural brucite and magnesia were applied as catalysts in catalytic ozonation of phenol in this work. It was found that both brucite and magnesia had remarkable accelerations on degradation of phenol and removal of COD in water. On this basis, effective and feasible routes for catalytic ozonation of phenol in water were proposed. The influence of initial pH value, radical scavengers and reaction temperature were investigated. The results revealed that there were different ozonation mechanisms in two systems: molecular ozone direct oxidation mechanism was proved in catalytic ozonation with brucite, and hydroxyl radical mechanism was demonstrated to play a main role in catalytic ozonation with magnesia. (C) 2008 Elsevier B.V. All rights reserved.
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