Journal
OPTICS LETTERS
Volume 40, Issue 17, Pages 4170-4173Publisher
Optica Publishing Group
DOI: 10.1364/OL.40.004170
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Funding
- Japan Society for the Promotion of Science (JSPS) Bilateral Program (Japan-France)
- Grants-in-Aid for Scientific Research [13J01123] Funding Source: KAKEN
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We developed a Raman optical activity (ROA) spectroscopic system with visible-excited coherent anti-Stokes Raman scattering (CARS). A supercontinuum within the visible region was generated with a photonic crystal fiber pumped with both 532 and 1064 nm excitation, generating a multiplexed CARS-ROA spectrum covering the whole fingerprint region. In visible excitation, the CARS-ROA spectrum of (-)-beta-pinene shows a higher contrast ratio of the chirality-induced signal to the achiral background than that of the previously reported near-infrared CARS-ROA spectrum. (C) 2015 Optical Society of America
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