Journal
APPLIED CATALYSIS B-ENVIRONMENTAL
Volume 165, Issue -, Pages 57-62Publisher
ELSEVIER
DOI: 10.1016/j.apcatb.2014.09.065
Keywords
ZIF-8; Palladium; Silver; Formic acid; Hydrogen storage
Funding
- National Natural Science Foundation of China [21201134]
- Natural Science Foundation of Jiangsu Province [BK20130370]
- Natural Science Foundation of Hubei Province [2013CFB288]
- Creative Research Groups of Hubei Province [2014CFA007]
- Large-scale Instrument and Equipment Sharing Foundation of Wuhan University
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Highly dispersed bimetallic AgPd nanoparticles with different composition have been successfully deposited on the metal-organic frameworks (ZIF-8) by using a simple liquid impregnation method. The resultant catalysts are composition dependent toward dehydrogenation of formic acid, while Ag18Pd82@ZIF-8 exhibits exceedingly high catalytic activity, with the turnover frequency (TOF) value of 580h(-1), and 100% hydrogen selectivity at 80 degrees C. (C) 2014 Elsevier B.V. All rights reserved.
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