4.7 Article

Atomically precise (catalytic) particles synthesized by a novel cluster deposition instrument

Journal

JOURNAL OF CHEMICAL PHYSICS
Volume 140, Issue 17, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.4871799

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Funding

  1. U.S. Department of Energy, BES-Materials Sciences [DE-AC-02-06CH11357]
  2. UChicago Argonne, LLC
  3. U.S. Department of Energy, Scientific User Facilities [DE-AC-02-06CH11357]

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We report a new high vacuum instrument which is dedicated to the preparation of well-defined clusters supported on model and technologically relevant supports for catalytic and materials investigations. The instrument is based on deposition of size selected metallic cluster ions that are produced by a high flux magnetron cluster source. The throughput of the apparatus is maximized by collecting and focusing ions utilizing a conical octupole ion guide and a linear ion guide. The size selection is achieved by a quadrupole mass filter. The new design of the sample holder provides for the preparation of multiple samples on supports of various sizes and shapes in one session. After cluster deposition onto the support of interest, samples will be taken out of the chamber for a variety of testing and characterization. (C) 2014 AIP Publishing LLC.

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