Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 140, Issue 6, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4863985
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Funding
- JSPS KAKENHI [24245003, 19002006, 24-4164, 24750011]
- Global COE Program (Chemistry Innovation through Cooperation of Science and Engineering)
- Special Coordination Funds for Promoting Science and Technology
- Grants-in-Aid for Scientific Research [24750011] Funding Source: KAKEN
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We report the observation of laser-assisted electron diffraction (LAED) through the collision of 1 keV electrons with gas-phase CCl4 molecules in a femtosecond near-infrared laser field. In the angular distribution of the scattered electrons with the energy shifts of +/-(h) over bar omega, we observed clear diffraction patterns which reflect the geometrical structure of the molecules at the moment of laser irradiation. Our results demonstrate that ultrafast nuclear dynamics of molecules can be probed by LAED with the high temporal (<10 fs) and spatial (similar to 0.01 angstrom) resolutions. (C) 2014 AIP Publishing LLC.
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