Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 139, Issue 7, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4818533
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Funding
- PIQA Program
- [CDCH-ULA-ADG-C09-95]
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We derive expressions for the transverse diffusion coefficient D(z) and the average persistence time tau(z; L) within a layer of width L, for particles of a non-homogeneous fluid enclosed in a planar nanopore. The method allows the direct evaluation of these position-dependent dynamical quantities from the equilibrium local particle density profile. We use results for the density and persistence time profiles from the virtual layer molecular dynamics method to numerically assess the significance of the Smoluchowski approximation. (C) 2013 AIP Publishing LLC.
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