Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 136, Issue 17, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4706899
Keywords
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Funding
- Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy
- National Science Foundation [CHE-1058791]
- National Institutes of Health [GM-59230]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1058791] Funding Source: National Science Foundation
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Expressions for the two-dimensional stimulated x-ray Raman spectroscopy (2D-SXRS) signal obtained using attosecond x-ray pulses are derived. The 1D- and 2D-SXRS signals are calculated for trans-N-methyl acetamide (NMA) with broad bandwidth (181 as, 14.2 eV FWHM) pulses tuned to the oxygen and nitrogen K-edges. Crosspeaks in 2D signals reveal electronic Franck-Condon overlaps between valence orbitals and relaxed orbitals in the presence of the core-hole. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4706899]
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