Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 137, Issue 8, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4746695
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- CNPq
- FAPERGS
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We provide extended evidence that mode-coupling theory (MCT) of supercooled liquids for the F-12 schematic model admits a microscopic realization based on facilitated spin models with tunable facilitation. Depending on the facilitation strength, one observes two distinct dynamical glass transition lines-continuous and discontinuous-merging at a dynamical tricritical-like point with critical decay exponents consistently related by MCT predictions. The mechanisms of dynamical arrest can be naturally interpreted in geometrical terms: the discontinuous and continuous transitions correspond to bootstrap and standard percolation processes, in which the incipient spanning cluster of frozen spins forms either a compact or a fractal structure, respectively. Our cooperative dynamical facilitation picture of glassy behavior is complementary to the one based on disordered systems and can account for higher-order singularity scenarios in the absence of a finite temperature thermodynamic glass transition. We briefly comment on the relevance of our results to finite spatial dimensions and to the F-13 schematic model. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4746695]
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