Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 133, Issue 16, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3495950
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Funding
- German-Israeli Foundation (GIF)
- DFG (Graduiertenkolleg) [GRK 1221]
- Studienstiftung des deutschen Volkes
- Harold Perlman Family
- EMALI network of the EU
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Recently we introduced the von Neumann representation as a joint time-frequency description for femtosecond laser pulses and suggested its use as a basis for pulse shaping experiments. Here we use the von Neumann basis to represent multidimensional molecular control landscapes, providing insight into the molecular dynamics. We present three kinds of time-frequency phase space scanning procedures based on the von Neumann formalism: variation of intensity, time-frequency phase space position, and/or the relative phase of single subpulses. The shaped pulses produced are characterized via Fourier-transform spectral interferometry. Quantum control is demonstrated on the laser dye IR140 elucidating a time-frequency pump-dump mechanism. (C) 2010 American Institute of Physics. [doi:10.1063/1.3495950]
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