Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 131, Issue 19, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3259653
Keywords
absorbing media; coherent antiStokes Raman scattering; multiwave mixing; optical materials; optical pulse generation
Funding
- NIGMS NIH HHS [GM-59230, R01 GM059230] Funding Source: Medline
- Direct For Mathematical & Physical Scien [0745892] Funding Source: National Science Foundation
- Division Of Chemistry [0745892] Funding Source: National Science Foundation
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A transition-amplitude based representation of heterodyne detected coherent anti-Stokes Raman signals is used to separate them into a parametric component that involves no change in the material and dissipative processes associated with various transitions between states. Qualitatively different contributions from the two processes are predicted for the signal generated by an overlapping narrow (picosecond) and broad-band (femtosecond) pulse.
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