Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 131, Issue 7, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3211305
Keywords
colloids; electrolytes; jellium; Monte Carlo methods; SCF calculations; suspensions; thermodynamics
Funding
- CNPq
- INCT-FCx of Brazil
- Air Force Office of Scientific Research (AFOSR), USA [FA9550-09-1-0283]
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An approach is proposed which allows to self-consistently calculate the structural and the thermodynamic properties of highly charged aqueous colloidal suspensions. The method is based on the renormalized jellium model with the background charge distribution related to the colloid-colloid correlation function. The theory is used to calculate the correlation functions and the effective colloidal charges for suspensions containing additional monovalent electrolyte. The predictions of the theory are in excellent agreement with Monte Carlo simulations.
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