Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 131, Issue 18, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3257678
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Funding
- Swedish Research Council (VR)
- Swedish Research Links MENA
- Goran Gustafsson Foundation (UU/KTH), Sweden
- Knut and Alice Wallenberg Foundation, Sweden
- AlbaNova Research Centre in Stockholm
- Italian Ministry for Research and University
- PRIN
- FIRB
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Conventional photoelectron and time-of-flight photoelectron-photoelectron coincidence (TOF-PEPECO) spectra have been measured for the outer valence region of the 1,4-bromofluorobenzene molecule. The photoelectron spectra were recorded using Hela radiation from a resonance Source, and the TOF-PEPECO spectra were recorded using HeII alpha radiation from a pulsed resonance source. The former provide energies of the cationic states and the latter of the dicationic states. The spectra are adequately interpreted with the aid of accurate Green's function calculations, showing very significant correlation effects. The lowest double ionization energy is found at 23.45 eV associated with the (4b(1))X-2 (1)A(1) dicationic state. (C) 2009 American Institute of Physics. [doi: 10.1063/1.3257678]
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