Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 130, Issue 5, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3068548
Keywords
coherent antiStokes Raman scattering; high-speed optical techniques; infrared spectra; nonlinear optics; optical frequency conversion; pulse shaping
Funding
- Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science
- U.S. Department of Energy
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Closed expressions are derived which incorporate pulse shaping effects in femtosecond nonlinear optical signals involving various combinations of temporally well-separated vibrationally resonant infrared and electronically off-resonant Raman pulses. Combinations of broadband and narrow band pulses that yield multidimensional extensions of coherent anti-Stokes Raman and sum frequency generation spectroscopy are presented.
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