Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 131, Issue 9, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3218843
Keywords
atom-molecule collisions; atom-molecule reactions; nitrogen; oxygen compounds; reaction kinetics theory; rotational-vibrational energy transfer; vibrational states
Funding
- Pole de Sciences Planetaires of Bourgogne Franche-Comte
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A detailed quasiclassical trajectory on the N+OH(v=0, j=0,1,5,10)-> NO+H reaction is reported at four collision energies from 0.01 to 0.5 eV. The vibrational distributions which are statistical and the angular distributions, which present a forward/backward symmetry, are consistent with the formation of a long-lived intermediate complex. Our results show globally a weak dependence of the angular and rovibrational distributions on the rotational excitation of OH, but a more pronounced effect of the collision energy.
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