Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 129, Issue 10, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.2973588
Keywords
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Funding
- Ministry of Education, Culture, Sports, Science and Technology, Japan
- Control of Molecules in Intense Laser Fields [14077205]
- 21st Century COE program for Frontiers in Fundamental Chemistry
- Specially Promoted Research on Ultrafast Hydrogen Migration [19002006]
- Global COE Program for Chemistry Innovation
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The ejection processes of hydrogen molecular ion H-3(+) from 12 kinds of hydrocarbon molecular species, methanol, ethanol, 1-propanol, 2-propanol, acetone, acetaldehyde, methane, ethane, ethylene, allene, 1,3-butadiene, and cyclohexane, induced by intense laser fields (similar to 10(14) W/cm(2)) have been investigated by time-of-flight mass spectroscopy. The observation of the H-3(+) production with the kinetic energy range of 3.5-5.0 eV from doubly ionized ethylene, allene, 1,3-butadiene, and cyclohexane, which have no methyl groups, showed the existence of the ultrafast hydrogen migration processes that enables three hydrogen atoms to come together to form H-3(+) within a hydrocarbon molecule. (c) 2008 American Institute of Physics.
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