Journal
JOURNAL OF CATALYSIS
Volume 284, Issue 2, Pages 157-164Publisher
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcat.2011.10.009
Keywords
Zeolite; Cu-ZSM-5; Dioxygen activation; Dicopper(II)-oxo; Selective methane oxidation; Bio-inorganic mimicking; C-H activation
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Funding
- Flemish Government
- NIH [DK-31450]
- Gerhard Casper Stanford Graduate Fellowship
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The present work highlights recent advances in elucidating the methane oxidation mechanism of the inorganic Cu-ZSM-5 biomimic and in identifying the reactive intermediates that are involved. Such molecular understanding is important in view of upgrading abundantly available methane, but also to comprehend the working mechanism of genuine Cu-containing oxidation enzymes. (C) 2011 Elsevier Inc. All rights reserved.
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