Journal
JOURNAL OF APPLIED PHYSICS
Volume 116, Issue 16, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4899190
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Funding
- NSF
- MOST of China
- US NSF PIRE (Partnership for International Research and Education) [OISE-0968226, DMR-1105961]
- JAEA Reimei Project at IOP, Columbia
- PSI
- McMaster
- TU Munich
- NSERC
- CIFAR at McMaster
- Office Of The Director
- Office Of Internatl Science &Engineering [0968226] Funding Source: National Science Foundation
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Here, we report the successful synthesis of a spin-and charge-decoupled diluted magnetic semiconductor (DMS) (Ca,Na)(Zn,Mn)(2)As-2, crystallizing into the hexagonal CaAl2Si2 structure. The compound shows a ferromagnetic transition with a Curie temperature up to 33 K with 10% Na doping, which gives rise to carrier density of n(p) similar to 10(20) cm(-3). The new DMS is a soft magnetic material with H-C < 400 Oe. The anomalous Hall effect is observed below the ferromagnetic ordering temperature. With increasing Mn doping, ferromagnetic order is accompanied by an interaction between the local spin and mobile charge, giving rise to a minimum in resistivity at low temperatures and localizing the conduction electrons. The system provides an ideal platform for studying the interaction of the local spins and conduction electrons. (C) 2014 AIP Publishing LLC.
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