4.6 Article

Enhancement of thermoelectric efficiency in a double-quantum-dot molecular junction

Journal

JOURNAL OF APPLIED PHYSICS
Volume 108, Issue 2, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.3457124

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Funding

  1. National Natural Science Foundation of China (NSFC) [10947130]
  2. Science Foundation of the Education Committee of Jiangsu Province [09KJB140001]
  3. Foundations of Changshu Institute of Technology

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We propose a high-efficiency molecular. junction consisting of a double-coupled-quantum-dot molecule sandwiched between two metallic electrodes. ZT can be enhanced in the Fano-line-shape regime, and it is sensitive to the magnetic flux threading through the double-coupled-quantum-dot molecular junction. This is mainly due to the local density of states in the Fano-line-shape regime may become narrower, and an abrupt changing in the conductance (transmission) spectrum is developed. We find the value of ZT can exceed 1 at room temperature by controlling the chemical potential or magnetic flux. So our results indicate such a molecular junction may be used to the solid-state thermoelectric energy-conversion device at room temperature. (C) 2010 American Institute of Physics. [doi: 10.1063/1.3457124]

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