Journal
NANOSCALE
Volume 7, Issue 39, Pages 16195-16199Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5nr03791c
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Funding
- National Science Foundation [ECCS0846018, ECCS0824186]
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The solution-processed PbSe colloidal quantum-dot (CQD) infrared photodetector with tandem architecture is proposed to address the high dark current issue. The electrical transport mechanism in tandem has been fundamentally changed in which the recombination of carriers at an intermediate layer becomes dominant rather than carriers hopping between nearest neighbors in CQD materials. As a result, the tandem photodetector exhibits ultra-high detectivities of 4.7 x 10(13) Jones and 8.1 x 10(13) Jones under 34 mu W cm(-2) illumination at 1100 nm, at 275 K and 100 K, respectively.
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